Magnetic structure of UPd2Si2

B. Shemirani, H. Lin, M. F. Collins, C. V. Stager, J. D. Garrett, and W. J. L. Buyers
Phys. Rev. B 47, 8672 – Published 1 April 1993
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Abstract

Elastic-neutron-scattering and magnetization measurements have been performed on a single crystal of UPd2Si2 in the 12–160-K temperature range. Two magnetically ordered phases are observed with the magnetic moment parallel to the c axis. At low temperatures (T<108 K), there is a simple body-centered-tetragonal antiferromagnet with an ordered moment of 2.3±0.3μB. At higher temperatures (108 K<T<136 K), there is an incommensurate spin-density wave with wave vector q=(0,0,0.732) and magnetic moment 2.3±0.3μB at 120 K. The phase transition at 108 K is first order while there is a critical phase transition at 136 K to the paramagnetic phase with critical index β=0.30±0.03. The low-temperature phase contains a small amount of a (0,0,2/3) phase; the maximum intensity from this phase is about 0.8% of that from the simple antiferromagnetic phases at 90 K. The magnetization in low field shows an analogous peak at 90 K.

  • Received 30 October 1992

DOI:https://doi.org/10.1103/PhysRevB.47.8672

©1993 American Physical Society

Authors & Affiliations

B. Shemirani, H. Lin, M. F. Collins, C. V. Stager, and J. D. Garrett

  • Department of Physics and Institute for Materials Research, McMaster University, Hamilton, Ontario, Canada L8S 4M1

W. J. L. Buyers

  • AECL Research, Chalk River, Ontario, Canada K0J 1J0

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Vol. 47, Iss. 14 — 1 April 1993

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