Low-energy plasmon excitations in infinite-layer nickelates

Luciano Zinni, Matías Bejas, Hiroyuki Yamase, and Andrés Greco
Phys. Rev. B 107, 014503 – Published 5 January 2023

Abstract

The discovery of superconductivity in infinite-layer nickelates is presently an important topic in condensed-matter physics, and potential similarities to and differences from cuprates are under intense debate. We determine general features of the charge excitation spectrum in nickelates from two opposite viewpoints: (i) Nickelates are regarded as strongly correlated electron systems like cuprate superconductors and thus can be described by the tJ model, and (ii) electron correlation effects are not as strong as in cuprates, and thus, random-phase approximation (RPA) calculations may capture the essential physics. We find that in both cases, plasmon excitations are realized around the momentum transfer q=(0,0,qz), although they tend to be damped more strongly in the RPA. In particular, this damping is enhanced by the relatively large interlayer hopping expected in nickelates. Besides reproducing the optical plasmon at q=(0,0,0) observed in Nd0.8Sr0.2NiO2, we obtain low-energy plasmons with gaps of 360 and 560 meV at q=(0,0,qz) for finite qz in cases (i) and (ii), respectively. The present work offers a possible theoretical hint to answer whether nickelates are cupratelike or not and contributes to the general understanding of the charge dynamics in nickelates.

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  • Received 28 July 2022
  • Revised 21 December 2022
  • Accepted 22 December 2022

DOI:https://doi.org/10.1103/PhysRevB.107.014503

©2023 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Luciano Zinni1, Matías Bejas2, Hiroyuki Yamase3, and Andrés Greco2

  • 1Facultad de Ciencias Exactas, Ingeniería y Agrimensura, Avenida Pellegrini 250, 2000 Rosario, Argentina
  • 2Facultad de Ciencias Exactas, Ingeniería y Agrimensura and Instituto de Física Rosario (UNR-CONICET), Avenida Pellegrini 250, 2000 Rosario, Argentina
  • 3International Center of Materials Nanoarchitectonics, National Institute for Materials Science, Tsukuba 305-0047, Japan

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Issue

Vol. 107, Iss. 1 — 1 January 2023

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