Thermal spin dynamics of Kitaev magnets: Scattering continua and magnetic field induced phases within a stochastic semiclassical approach

Oliver Franke, Dumitru Călugăru, Andreas Nunnenkamp, and Johannes Knolle
Phys. Rev. B 106, 174428 – Published 21 November 2022

Abstract

The honeycomb magnet αRuCl3 is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS) response at finite frequency has been interpreted as that of a “proximate QSL.” A moderate in-plane magnetic field indeed melts the residual zigzag order, giving rise to peculiar intermediate-field phases before the high-field polarized state. In INS measurements the low-frequency spin waves disappear, leading to a broad scattering continuum in the field-induced intermediate regime, whose nature is currently under debate. Here, we study the magnetic-field-dependent spin dynamics of the KΓΓ model within a stochastic semiclassical treatment, which incorporates the effect of finite-temperature fluctuations. At temperatures relevant for INS experiments, we show how the excitations of the zigzag phase broaden and that the different intermediate phases all show a similar continuum response. We discuss the implications of our results for experiments and highlight the importance of distinguishing finite-temperature fluctuations from genuine quantum fractionalization signatures in frustrated magnets.

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  • Received 11 July 2022
  • Revised 29 September 2022
  • Accepted 7 November 2022

DOI:https://doi.org/10.1103/PhysRevB.106.174428

©2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Oliver Franke1,2,*, Dumitru Călugăru3,4,*, Andreas Nunnenkamp5,4, and Johannes Knolle1,6,7

  • 1Department of Physics TQM, Technische Universität München, James-Franck-Straße 1, D-85748 Garching, Germany
  • 2Dahlem Center for Complex Quantum Systems and Physics Department, Freie Universität Berlin, Arnimallee 14, 14195 Berlin, Germany
  • 3Department of Physics, Princeton University, Princeton, New Jersey 08544, USA
  • 4Cavendish Laboratory, University of Cambridge, Cambridge CB3 0HE, United Kingdom
  • 5Faculty of Physics, University of Vienna, Boltzmanngasse 5, 1090 Vienna, Austria
  • 6Munich Center for Quantum Science and Technology (MCQST), 80799 Munich, Germany
  • 7Blackett Laboratory, Imperial College London, London SW7 2AZ, United Kingdom

  • *These authors contributed equally to this work.

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Issue

Vol. 106, Iss. 17 — 1 November 2022

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