Synthetic antiferromagnets (SAFs) with perpendicular magnetic anisotropy (PMA) have recently attracted intensive attention for their potential applications in domain-wall-based racetrack memory. In this paper, swift heavy Fe ion irradiation is introduced to tune the magnetic properties of Pt/Co/Pt/Ru/Pt/Co/Ta SAFs from spin-flip to spin-flop transition. The evolutions of magnetic domain and domain wall motion are investigated to obtain the microscopic insight into the change of magnetic states. Both the experimental and the simulated results demonstrate that different responses of the effective PMA constant and the interlayer-exchange-coupling strength to ion irradiation determine the magnetic-phase transitions. The structure evolution from experiments and theoretical simulations suggests that the ion-irradiation-induced damage mainly happens at the Pt/Co interface. The damage leads to the different decrease rates of the effective PMA constant and the interlayer-exchange-coupling strength due to their intrinsic direct and Ruderman-Kittel-Kasuya-Yosida interaction nature, respectively. A quite good thermal stability of samples is obtained with ion fluence $<1.5\times {10}^{14}\mathrm{ions}/\mathrm{c}{\mathrm{m}}^2$. In this paper, we demonstrate that ion irradiation is a promising method to tailor magnetic properties of SAFs. Additionally, the ion-irradiation-induced well-controlled antiferromagnetically coupled domains could show potential applications in spintronic devices.

• Received 15 June 2021
• Revised 23 September 2021
• Accepted 28 September 2021

DOI:https://doi.org/10.1103/PhysRevB.104.134416