Abstract
We have studied the magnetization process of the new insulating ferromagnetic semiconductor (Al,Fe)Sb by means of x-ray magnetic circular dichroism. For an optimally doped sample with 10% Fe, a magnetization was found to rapidly increase at low magnetic fields and to saturate at high magnetic fields at room temperature, well above the Curie temperature of 40 K. We attribute this behavior to the existence of nanoscale Fe-rich ferromagnetic domains acting as superparamagnets. By fitting the magnetization curves using the Langevin function representing superparamagnetism plus the paramagnetic linear function, we estimated the average magnetic moment of the nanoscale ferromagnetic domain to be and the fraction of Fe atoms participating in the nanoscale ferromagnetism to be . Such behavior was also reported for (In,Fe)As:Be and Ge:Fe and seems to be a universal characteristic of the Fe-doped ferromagnetic semiconductors. Further Fe doping up to 14% led to the weakening of the ferromagnetism, probably because antiferromagnetic superexchange interaction between nearest-neighbor Fe-Fe pairs becomes dominant.
- Received 11 February 2019
- Revised 17 October 2019
- Accepted 27 January 2020
- Corrected 12 May 2020
DOI:https://doi.org/10.1103/PhysRevB.101.075204
©2020 American Physical Society
Physics Subject Headings (PhySH)
Corrections
12 May 2020
Correction: The order of authors has been modified, and the affiliations are now identified by superscript numbers. A second affiliation has been added for the last author.