Near-infrared resonance-mediated chirp control of a coherently generated broadband deep-ultraviolet spectrum

Leonid Rybak, Lev Chuntonov, Andrey Gandman, Naser Shakour, and Zohar Amitay
Phys. Rev. A 84, 035401 – Published 12 September 2011

Abstract

We investigate the use of shaped near-infrared (NIR) femtosecond pulses to control the generation of coherent broadband deep-ultraviolet (DUV) radiation in an atomic resonance-mediated (2+1) three-photon excitation to a broad far-from-resonance continuum. Previously, we have shown control over the total emitted DUV yield. Here, we experimentally demonstrate phase control over the spectral characteristics (central frequency and bandwidth) of the emitted broadband DUV radiation. It is achieved by tuning the linear chirp applied to the exciting NIR femtosecond pulse. The study is conducted with Na vapor.

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  • Received 15 June 2011

DOI:https://doi.org/10.1103/PhysRevA.84.035401

©2011 American Physical Society

Authors & Affiliations

Leonid Rybak, Lev Chuntonov*, Andrey Gandman, Naser Shakour, and Zohar Amitay

  • The Shirlee Jacobs Femtosecond Laser Research Laboratory, Schulich Faculty of Chemistry, Technion - Israel Institute of Technology, Haifa 32000, Israel

  • *Present address: Department of Chemical Physics, Weizmann Institute of Science, Rehovot 76100, Israel.
  • Present address: Department of Chemistry, University of California, Berkeley, CA 94720, USA.
  • amitayz@technion.ac.il

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Vol. 84, Iss. 3 — September 2011

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