Soft-sphere model for the glass transition in binary alloys. II. Relaxation of the incoherent density-density correlation functions

G. Pastore, B. Bernu, J. P. Hansen, and Y. Hiwatari
Phys. Rev. A 38, 454 – Published 1 July 1988
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Abstract

Using molecular-dynamics (MD) data on a binary-alloy model, we have computed the self (incoherent) -part of the density autocorrelation functions of both species in the supercooled liquid and near the glass transition, over an extensive range of wave numbers. Standard theoretical models of liquid-state theory fail to reproduce the data, while the Chudley-Elliott jump diffusion model yields reasonable results in the glass range. With a suitable scaling of the time axis, the data for different temperatures can be brought onto a single master curve, which is well fitted by a Kohlrausch (‘‘stretched-exponential’’) function with a wave-number-dependent exponent.

  • Received 27 January 1988

DOI:https://doi.org/10.1103/PhysRevA.38.454

©1988 American Physical Society

Authors & Affiliations

G. Pastore

  • International School for Advanced Studies, Strada Costiera 11, I-34014 Trieste, Italy

B. Bernu

  • Laboratoire de Physique Théorique des Liquides, Université Pierre et Marie Curie, 75252 Paris Cédex 05, France

J. P. Hansen

  • Laboratoire de Physique, Ecole Normale Supérieure de Lyon, 69364 Lyon Cédex 07, France

Y. Hiwatari

  • Department of Physics, Faculty of Science, Kanazawa University, Marunouchi 1-1, Kanazawa, Ishikawa 920, Japan

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Vol. 38, Iss. 1 — July 1988

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