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Cooper minimum of high-order harmonic spectra from an MgO crystal in an ultrashort laser pulse

Yiting Zhao, Xiaoqin Xu, Shicheng Jiang, Xi Zhao, Jigen Chen, and Yujun Yang
Phys. Rev. A 101, 033413 – Published 25 March 2020

Abstract

Cooper minimum structure of high-order harmonic spectra from atoms or molecules has been extensively studied. In this paper, we demonstrate that the crystal harmonic spectra from an ultrashort midinfrared laser pulse also exhibit the Cooper minimum characteristic. Based on the accurate band dispersion and k-dependent transition dipole moment (TDM) from the first-principles calculations, it can be found that the harmonic spectra from the MgO crystal along the ΓX direction present a dip structure in the plateau, which is originated from the valley of TDM by examining the distribution of the harmonic intensity at the k space. The Cooper minimum feature in crystal high-order-harmonic generation (HHG) will pave a new way to retrieve the band information of solid materials by using HHG from the ultrashort midinfrared laser pulse.

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  • Received 19 September 2019
  • Accepted 2 March 2020

DOI:https://doi.org/10.1103/PhysRevA.101.033413

©2020 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Yiting Zhao1,2, Xiaoqin Xu1, Shicheng Jiang3, Xi Zhao4, Jigen Chen1,*, and Yujun Yang2,†

  • 1Zhejiang Provincial Key Laboratory for Cutting Tools, Taizhou University, Taizhou 31800, China
  • 2Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China
  • 3State Key Laboratory of Precision Spectroscopy, East China Normal University, Shanghai 200062, China
  • 4Department of Physics, J. R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas 66506, USA

  • *kiddchen@126.com
  • yangyj@jlu.edu.cn

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Issue

Vol. 101, Iss. 3 — March 2020

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