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Effect of Surface Elasticity on the Rheology of Nanometric Liquids

Richard Villey, Emmanuelle Martinot, Cécile Cottin-Bizonne, Magali Phaner-Goutorbe, Liliane Léger, Frédéric Restagno, and Elisabeth Charlaix
Phys. Rev. Lett. 111, 215701 – Published 20 November 2013
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Abstract

The rheological properties of liquids confined to nanometer scales are important in many physical situations. In this Letter, we demonstrate that the long-range elastic deformation of the confining surfaces must be taken into account when considering the rheology of nanometric liquids. In the case of a squeeze-flow geometry, we show that below a critical distance Dc, the liquid is clamped by its viscosity and its intrinsic properties cannot be disentangled from the global system response. Using nanorheology experiments, we demonstrate that picometer elastic deflections of the rigid confining surfaces dominate the overall mechanical response of nanometric liquids confined between solid walls.

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  • Received 6 June 2013

DOI:https://doi.org/10.1103/PhysRevLett.111.215701

© 2013 American Physical Society

Authors & Affiliations

Richard Villey1, Emmanuelle Martinot2, Cécile Cottin-Bizonne1, Magali Phaner-Goutorbe3, Liliane Léger2, Frédéric Restagno2,*, and Elisabeth Charlaix4,†

  • 1Institut Lumière Matière, Université Lyon 1, CNRS, F-69622 Villeurbanne, France
  • 2Laboratoire de physique des solides, Université Paris-Sud CNRS, F-91405 Orsay, France
  • 3Institut des Nanotechnologies de Lyon, École Centrale de Lyon, CNRS, Université de Lyon, F-69134 Ecully, France
  • 4Laboratoire interdisciplinaire de physique, Université Grenoble 1, CNRS, F-38402 Grenoble, France

  • *frederic.restagno@u-psud.fr
  • elisabeth.charlaix@ujf-grenoble.fr

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Issue

Vol. 111, Iss. 21 — 22 November 2013

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