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Direct observation of Fe spin reorientation in single-crystalline YbFe6Ge6

M A Avila et al 2005 J. Phys.: Condens. Matter 17 6969-6979   doi: 10.1088/0953-8984/17/43/014  Help

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M A Avila1, T Takabatake1, Y Takahashi2, S L Bud'ko3 and P C Canfield3
1 Department of Quantum Matter, ADSM, Hiroshima University, Higashi-Hiroshima 739-8530, Japan
2 Department of Earth and Planetary Systems Sciences, Hiroshima University, Higashi-Hiroshima 739-8526, Japan
3 Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, IA 50011, USA

Abstract. We have grown single crystals of YbFe6Ge6 and LuFe6Ge6 and characterized their anisotropic behaviour through low-field magnetic susceptibility, field-dependent magnetization, resistivity and heat capacity measurements. The Yb3+ valency is confirmed by LIII XANES measurements. YbFe6Ge6 crystals exhibit a field-dependent, sudden reorientation of the Fe spins at about 63 K, a unique effect in the RFe6Ge6 family (R =  rare earths), where the Fe ions order anti-ferromagnetically with Neél temperatures above 450 K and the R ions' magnetism appears to behave independently. The possible origins of this unusual behaviour of the ordered Fe moments in this compound are discussed.

Print publication: Issue 43 (2 November 2005)
Received 16 August 2005, in final form 25 September 2005
Published 14 October 2005

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