Issue 20, 2023

Porous crystalline materials for memories and neuromorphic computing systems

Abstract

Porous crystalline materials usually include metal–organic frameworks (MOFs), covalent organic frameworks (COFs), hydrogen-bonded organic frameworks (HOFs) and zeolites, which exhibit exceptional porosity and structural/composition designability, promoting the increasing attention in memory and neuromorphic computing systems in the last decade. From both the perspective of materials and devices, it is crucial to provide a comprehensive and timely summary of the applications of porous crystalline materials in memory and neuromorphic computing systems to guide future research endeavors. Moreover, the utilization of porous crystalline materials in electronics necessitates a shift from powder synthesis to high-quality film preparation to ensure high device performance. This review highlights the strategies for preparing porous crystalline materials films and discusses their advancements in memory and neuromorphic electronics. It also provides a detailed comparative analysis and presents the existing challenges and future research directions, which can attract the experts from various fields (e.g., materials scientists, chemists, and engineers) with the aim of promoting the applications of porous crystalline materials in memory and neuromorphic computing systems.

Graphical abstract: Porous crystalline materials for memories and neuromorphic computing systems

Article information

Article type
Review Article
Submitted
17 Aug 2023
First published
27 Sep 2023

Chem. Soc. Rev., 2023,52, 7071-7136

Porous crystalline materials for memories and neuromorphic computing systems

G. Ding, J. Zhao, K. Zhou, Q. Zheng, S. Han, X. Peng and Y. Zhou, Chem. Soc. Rev., 2023, 52, 7071 DOI: 10.1039/D3CS00259D

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