Issue 34, 2021

High optoelectronic performance of a local-back-gate ReS2/ReSe2 heterojunction phototransistor with hafnium oxide dielectric

Abstract

A high optoelectronic performance ReS2/ReSe2 van der Waals (vdW) heterojunction phototransistor utilizing thin hafnium oxide (HfO2) as a local-back-gate dielectric layer was prepared and studied. The heterojunction-based phototransistor exhibits a superior electrical performance with a large rectification ratio of ∼103. Furthermore, unlike diode-like heterojunction devices, the innovative introduction of a local-back-gate in this phototransistor provides an outstanding gate-tunable capability with an ultra-low off-state current of 433 fA and a high on/off current ratio of over 106. And under optical excitation of a wide spectrum from 400 to 633 nm, an excellent photodetection responsivity at the 104 A W−1 level and the maximum normalized detectivity of 1.8 × 1015 Jones @ 633 nm have been demonstrated. Such high performances are attributed to the band alignment of the type-II heterojunction and the suppression of dark current by the local-back-gate. This work provides a promising reference for two-dimensional (2D) Re-based heterojunction optoelectronic devices.

Graphical abstract: High optoelectronic performance of a local-back-gate ReS2/ReSe2 heterojunction phototransistor with hafnium oxide dielectric

Article information

Article type
Paper
Submitted
29 Apr 2021
Accepted
21 Jul 2021
First published
21 Jul 2021

Nanoscale, 2021,13, 14435-14441

High optoelectronic performance of a local-back-gate ReS2/ReSe2 heterojunction phototransistor with hafnium oxide dielectric

Y. Li, X. Li, G. Zeng, Y. Chen, D. Chen, B. Peng, L. Zhu, D. W. Zhang and H. Lu, Nanoscale, 2021, 13, 14435 DOI: 10.1039/D1NR02728J

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