Issue 34, 2019

Laser-induced photoresistance effect in Si-based vertical standing MoS2 nanoplate heterojunctions for self-powered high performance broadband photodetection

Abstract

MoS2 has attracted extensive attention as the basic configuration of optoelectronic systems because of its outstanding optical and electronic properties. Although high performance MoS2-based photodetectors have been realized by many groups, these studies are still in their initial stages of research, and more importantly, the usual photocurrent or photovoltage signals are fundamentally susceptible, thus seeking novel structures or working principle devices becomes more fascinating. Here, the MoS2/Si heterojunction is prepared with a vertically standing nanoplate structure and we exploit it as a photovoltage, photocurrent and photoresistance-based multifunctional self-powered position sensitive detector (PSD). The PSD exhibits unprecedented performance with very high sensitivity (391.1 mV mm−1, 285.2 μA mm−1, and 21.61 KΩ mm−1 for photovoltage, photocurrent and photoresistance responses, respectively), excellent linearity (nonlinearity <2%), and a very fast response speed (4.75 ms/6.33 ms), all of which are much better than those obtained in many other systems. More importantly, it is the first time that lateral photoresistance (LPRE) is observed in a MoS2/Si heterojunction. Based on the theoretical analysis of the scattering or transportation modulation of photo-generated carriers on the drifted carriers in the MoS2/Si heterojunction, these results are well explained.

Graphical abstract: Laser-induced photoresistance effect in Si-based vertical standing MoS2 nanoplate heterojunctions for self-powered high performance broadband photodetection

Article information

Article type
Paper
Submitted
27 Jun 2019
Accepted
02 Aug 2019
First published
02 Aug 2019

J. Mater. Chem. C, 2019,7, 10642-10651

Laser-induced photoresistance effect in Si-based vertical standing MoS2 nanoplate heterojunctions for self-powered high performance broadband photodetection

S. Qiao, J. Liu, G. Fu, S. Wang, K. Ren and C. Pan, J. Mater. Chem. C, 2019, 7, 10642 DOI: 10.1039/C9TC03454D

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