Issue 8, 2018, Issue in Progress

Spin-dependent and spin-independent channels of electrical transport in perovskite manganites

Abstract

A model with two channels of electrical transport (TCET) for perovskite manganites is proposed, and it is described by an equivalent device with two current-carrier channels. In one channel, there is a spin-independent resistor (R3) with an equivalent resistivity of ρ3. In the other channel, there are two spin-dependent resistors in series (R1 and R2) with an equivalent resistivity of ρ1 + ρ2. The component ρ1 includes residual resistivity and the resistivity contributed by crystal-lattice scattering. The other component of the equivalent resistivity, ρ2, originates from the spin orientations of the itinerant electrons and the local electrons of the outer O 2p and Mn 3d orbits that deviate from the orientation of their ground states when the test temperature is close to the Curie temperature. Using this model, we fitted the experimental curves of the resistivity versus test temperature for single-crystalline La1−xSrxMnO3 (0.00 ≤ x ≤ 0.40) and polycrystalline La0.6Sr0.4Mn1−xFexO3 (0.00 ≤ x ≤ 0.30). In addition, we investigated the effects of the fraction of the antiferromagnetic phase, scattering at the crystallite interfaces, and the crystal-cell constants on the samples' resistivity. The physical mechanism of the TCET model was explained using an O 2p itinerant-electron model, which has been used in other studies to explain the magnetic ordering of several series of spinel ferrites and perovskite manganites.

Graphical abstract: Spin-dependent and spin-independent channels of electrical transport in perovskite manganites

Article information

Article type
Paper
Submitted
29 Nov 2017
Accepted
17 Jan 2018
First published
24 Jan 2018
This article is Open Access
Creative Commons BY-NC license

RSC Adv., 2018,8, 4417-4425

Spin-dependent and spin-independent channels of electrical transport in perovskite manganites

J. J. Qian, W. H. Qi, Z. Z. Li, L. Ma, G. D. Tang, Y. N. Du, M. Y. Chen, G. H. Wu and F. X. Hu, RSC Adv., 2018, 8, 4417 DOI: 10.1039/C7RA12878A

This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence. You can use material from this article in other publications, without requesting further permission from the RSC, provided that the correct acknowledgement is given and it is not used for commercial purposes.

To request permission to reproduce material from this article in a commercial publication, please go to the Copyright Clearance Center request page.

If you are an author contributing to an RSC publication, you do not need to request permission provided correct acknowledgement is given.

If you are the author of this article, you do not need to request permission to reproduce figures and diagrams provided correct acknowledgement is given. If you want to reproduce the whole article in a third-party commercial publication (excluding your thesis/dissertation for which permission is not required) please go to the Copyright Clearance Center request page.

Read more about how to correctly acknowledge RSC content.

Social activity

Spotlight

Advertisements