Issue 20, 2016

Polarization conversion-based molecular sensing using anisotropic plasmonic metasurfaces

Abstract

Anisotropic media induce changes in the polarization state of transmitted and reflected light. Here we combine this effect with the refractive index sensitivity typical of plasmonic nanoparticles to experimentally demonstrate self-referenced single wavelength refractometric sensing based on polarization conversion. We fabricated anisotropic plasmonic metasurfaces composed of gold dimers and, as a proof of principle, measured the changes in the rotation of light polarization induced by biomolecular adsorption with a surface sensitivity of 0.2 ng cm−2. We demonstrate the possibility of miniaturized sensing and we show that experimental results can be reproduced by analytical theory. Various ways to increase the sensitivity and applicability of the sensing scheme are discussed.

Graphical abstract: Polarization conversion-based molecular sensing using anisotropic plasmonic metasurfaces

Supplementary files

Article information

Article type
Communication
Submitted
16 Feb 2016
Accepted
26 Apr 2016
First published
26 Apr 2016

Nanoscale, 2016,8, 10576-10581

Polarization conversion-based molecular sensing using anisotropic plasmonic metasurfaces

R. Verre, N. Maccaferri, K. Fleischer, M. Svedendahl, N. Odebo Länk, A. Dmitriev, P. Vavassori, I. V. Shvets and M. Käll, Nanoscale, 2016, 8, 10576 DOI: 10.1039/C6NR01336H

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