Abstract
Considerable theoretical and experimental work has lately been focused on waves localized in time and space. In optics, waves of that nature are often referred to as light bullets. The most fascinating feature of light bullets is their propagation without appreciable distortion by diffraction or dispersion. Here, analytic expressions for the fields of an ultra-short, tightly-focused and arbitrary-order Bessel pulse are derived and discussed. Propagation in an under-dense plasma, responding linearly to the fields of the pulse, is assumed throughout. The derivation stems from wave equations satisfied by the vector and scalar potentials, themselves following from the appropriate Maxwell equations and linked by the Lorentz gauge. It is demonstrated that the fields represent well a pulse of axial extension, L, and waist radius at focus, w0, both of the order of the central wavelength λ0. As an example, to lowest approximation, the pulse of order l = 2 is shown to propagate undistorted for many centimeters, in vacuum as well as in the plasma. As such, the pulse behaves like a “light bullet” and is termed a “Bessel-Bessel bullet of arbitrary order”. The field expressions will help to better understand light bullets and open up avenues for their utility in potential applications.
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Introduction
Bessel beams were discovered more than three decades ago1,2 and have found numerous applications since, such as in optical trapping and tweezing3,4,5,6, precision drilling7,8, optical microscopy9 and laser acceleration10. Tightly-focused and temporally short pulses (or equivalently, ones that are of finite spatial extensions) are currently in great demand for many applications11,12,13,14,15,16. Central to the utility of such pulses is the need for analytic expressions for their electric and magnetic field components.
This paper aims to present analytic expressions for the fields of an ultra-short and tightly-focused Bessel pulse of arbitrary order, propagating in an under-dense plasma. The expressions, essentially describing a non-spreading wavepacket17,18,19,20,21, can be useful for many applications, including laser acceleration and high-harmonic generation (HHG) by colliding a tightly-focused and ultra-short pulse with a counter-propagating electron bunch22. In particular, a non-spreading wavepacket is highly desirable for laser-assisted atomic HHG23,24,25. Other plasma-based applications, such as the creation of plasma channels26,27,28,29 treated theoretically by particle-in-cell (PIC) simulations, may find the analytic expressions quite useful.
This work introduces orbital angular momentum into the description of a bessel-Bessel bullet30,31, for the first time. Among other things, opening up the Hilbert space of orbital angular momentum to be used to encode information in the fields of the bullets will boost efforts to utilize them in information transfer32.
Laser Bessel beam technology, based upon the use of axicon lenses, or combinations of annular slits and Fourier transforming lenses2,32 to achieve the required polarizations, is quite established now. However, experimental realization of the specific orbital angular momentum states of a Bessel-Bessel bullet may be challenging. Attempts to produce spatio-temporally localized Bessel-Bessel bullets experimentally may be guided by, and can benefit from, the recent work of Wise et al.33 on Bessel-Airy light bullets.
The basic assumption made in this work is that the response of the plasma to the fields of the laser pulse may be considered linear34. This can reliably be the case for non-relativistic pulse peak intensities (roughly, as long as I ≪ 1018 W/cm2, for a laser wavelength of 1 μm). Under these conditions, Maxwell’s equations are entirely equivalent to30,35,36,37
for the vector potential A, together with a similar equation holding for the scalar potential, Φ, provided the two potentials are linked by the Lorentz gauge condition. Equation (1) has an effective plasma wavenumber kp = ωp/c, in which c is the speed of light in vacuum and the plasma frequency is \({\omega }_{p}=\sqrt{{n}_{0}{e}^{2}/m{\varepsilon }_{0}}\), where n0 is the number density of the ambient electrons, ε0 is the permittivity of free-space and m and −e are the mass and charge, respectively, of the electron.
Methods
Change of coordinates
Equation (1) will be solved for the vector potential and the Lorentz condition will be used to obtain the associated scalar potential30,31,37,38,39,40,41,42. This process finally culminates in finding expressions for the E and B fields from the space- and time-derivatives of the potentials35. First, the Laplacian is expressed in cylindrical coordinates (r, θ, z). Next, assuming propagation along the z-axis, the following pair of new coordinates will be introduced in terms of the z- coordinate and the time
For the centroid of the pulse (assumed to have been created at the origin of coordinates at t = 0 and to travel along the z- axis at approximately the speed of light) z ~ ct and, hence, η ~ ct and ζ ~ 0. In other words, η gives the position, on the propagation axis, of the centroid of the pulse at any time t, relative to the origin and ζ determines its coordinate relative to the moving centroid itself37. Employing the new variables, Eq. (1) transforms into
The fields to be derived below possess radially- as well as azimuthally-polarized electric field components. Thus, the object to be described by these fields will be an ultra-short and tightly-focused laser pulse, which carries orbital angular momentum. In other words, it is the ultra-short, tightly-focused analogue of an arbitrary-order Bessel beam1,2,32,42,43,44,45.
Truncated series solution
Letting \(\hat{z}\) be a unit vector in the propagation direction and k0 = 2π/λ0 a central wavenumber corresponding to a central wavelength λ0, a one-component vector potential is put forth through the ansatz42
with a0 a constant amplitude. The amplitude a(r, θ, η, ζ) is next synthesized from the Fourier components
Using Eqs (4) and (5) in (3) yields an equation30,31,37,40,41
for each Fourier component ak. Solution to Eq. (6) will be sought using the standard textbook technique of separation of the variables. Thus, inserting ak(r, θ, η, k) = fkF(r)Θ(θ)G(η) into (6) and separating the variables, as usual, gives
Solutions to the above equations, which describe the physical situation of interest to us in this work, are: Θ ~ exp(ilθ) with l an integer, G a simple complex exponential and F ~ Jl(krr) an ordinary Bessel function of the first kind and order l. Furthermore, kr is a separation constant, or radial index (not a radial wavenumber, because the wavevector does not have a radial component). In an experiment, the size of kr will ultimately be determined by the size of the aperture used to produce the pulse, as will be described below.
The kth Fourier component of the vector potential amplitude now takes on the form
with fk independent of η, θ and r. For fk, we make the simple choice46
Implied in this choice is the assumption that the initial wavepacket, which evolves into the propagating pulse, consists of waves that possess a uniform spectrum, or distribution of wavenumbers30,31,40 of width Δk and height \(\sqrt{2\pi }/{\rm{\Delta }}k\). Note that this choice renders ak(0,0,0,k) = fk. Strictly speaking, this holds only for l = 0, in which case fk has the Fourier transform a(0,0,0,ζ) = f(ζ) = sinc(ζΔk/2). The quantity | f(ζ)|2 represents the initial pulse intensity profile, with an approximate full-width-at-half-maximum ~2π/Δk. Thus, it is plausible to adopt L = 2π/Δk as representing the initial length (spatial extension) of the pulse in its propagation direction. On the other hand, the waist radius at focus, w0, will be shown shortly to be fixed by x1,l, the first zero of Jl.
Putting (9) into (8) and the result back into (5) gives
Unfortunately, the integration in (10) cannot be carried out in closed analytic form. However, viewed as a function of k′ = k + k0, ϕk can be power-series expanded around k0, according to
The integration in (10) may now be carried out in terms of incomplete gamma functions. Furthermore, on account of the fact that only the leading term(s) in (11) may contribute significantly in applications of interest, the series giving the full vector potential can be truncated to order n and written as
in which Δk has been replaced by 2π/L.
Zeroth-order vector potential
From A(n) follows a complete description for the fields of the ultra-short and tightly-focused pulse. The presence of Jl suggests that this object is the short-pulse analogue of an lth-order Bessel beam. The assumption will also be made that the first term in the series contributes the most, while terms beyond the first contribute negligibly30. Otherwise, one may still work with the truncated series to any desired order. The following expression for the zeroth-order vector potential follows from Eq. (12)
where the sinc function has been replaced by j0, the zero-order spherical Bessel function of the first kind, and φ0 is a constant phase. Note that in the case of a pulse containing a few cycles, φ0 plays the role of a carrier envelope phase (CEP).
For a pulse created at t = 0, with its centroid at the origin of coordinates, \({|{A}^{\mathrm{(0)}}/{a}_{0}|}^{2}={J}_{l}^{2}({k}_{r}r)\). Surface plots of this quantity, in the focal plane, are shown in Fig. 1, for l = 0, 1, 2 and 5, exhibiting all the expected properties of the square of Jl. It should also be borne in mind that the axial extension of the pulse, L, was determined above by the first zero of j0. The temporal width of the pulse may be taken as τ ~ L/c, while the waist radius at focus, w0, is such that krw0 = x1,l, the first zero of Jl. With the waist radius predetermined as w0 = 0.8λ0 in Figs 1–4, the radial index kr → kr,l, i.e., it takes on different values for the different orbital angular momentum states indexed by l. In an experiment, the radial indices and waist radii may alternatively be determined from knowledge of the radius ra of the aperture employed to produce and observe the intensity patterns. The radius wn containing the nth observed ring would be such that kr,lwn = xn,l, where xn,l is the nth zero of Jl. Using wn ~ ra, one gets kr,l ~ xn,l/ra. Had Fig. 1, in which ra = 3λ0, been produced experimentally, this procedure would have resulted in the values listed in the third column of Table 1 for the patterns displayed, respectively, in Fig. 1(a–d). These radial index values lead to the waist radii at focus listed in the fourth column of the same Table.
It will be demonstrated below that both L and w0 stay roughly fixed in magnitude during propagation of the pulse, thus making the pulse essentially diffraction-free and dispersion-free. This may all be traced back to the absence of nonlinear terms in Eq. (1). The above features qualify the pulse for being a “light bullet”33,46,47,48,49,50,51,52.
Results
The fields
The electric and magnetic fields of the pulse, explicit knowledge of which is required for many analytic and numerical calculations, follow from E = −∇Φ − ∂A/∂t and B = ∇ × A, most appropriately in cylindrical coordinates. The electric field has three components: radial Er, azimuthal Eθ and axial Ez. These may, respectively, be found from31,37
where s = ick0 − (1/a)∂a/∂t. Moreover, the magnetic field has two components: radial, Br and azimuthal, Bθ, which follow, respectively, from
According to Eqs (14–16) the electric field components, after some tedious algebra and with arguments of all the Bessel functions temporarily suppressed, are
Furthermore, Eq. (17) give the following expressions for the associated magnetic field components
In Eqs (18)–(22) E0 = ck0a0, and
Equations (18–24) give the field components of a pulse propagating in vacuum by taking the limit kp → 0. They also have the expected limits in the case of a zero-order Bessel pulse36, for which the components \({E}_{\theta }^{\mathrm{(0)}}\) and \({B}_{r}^{\mathrm{(0)}}\) are absent, while \({E}_{r}^{\mathrm{(0)}}\) and \({B}_{\theta }^{\mathrm{(0)}}\) vanish identically at all points on the z- axis. These components have the hollow intensity profiles displayed in Figs 2 and 3. Note also that for the l = 1 pulse only the intensity profile corresponding to \({E}_{z}^{\mathrm{(0)}}\) is hollow. On the other hand, all profiles are hollow for l ≥ 2, due to the vanishing of Jl at r = 0, for all l ≥ 1.
Propagation characteristics
Using the second of Eq. (13) one gets a general expression for the wavevector of the pulse in cylindrical coordinates, namely
According to Eq. (25) the wavevector does not have a radial component and wavefronts (surfaces of constant phase) are helices of fixed radii r. In this sense the bullet carries orbital angular momentum, with the index l labeling different states in the relevant Hilbert space42. In general, an effective frequency for the bullet may be obtained from ω = −∂φ(0)/∂t = c(k0 + α/2), from which the dispersion relation \({(\omega /c)}^{2}-{k}_{z}^{2}=2{k}_{0}\alpha \), follows immediately. From this, in turn, one gets an effective wavenumber \(k=\omega /c=\sqrt{{k}_{z}^{2}+{k}_{r}^{2}+{k}_{p}^{2}}\). For the fields to describe a propagating pulse, the axial wavevector must be positive definite, kz > 0. According to the last of Eqs. (25) this condition is equivalent to the requirement kr < 2k0 = 4π/λ0. All cases in Table 1 satisfy this condition and, hence, should describe pulses propagating through an aperture of radius ra = 3λ0.
Key propagation characteristics of the pulse are illustrated in Fig. 4. The figure displays surface plots, in the z-r plane, of the intensity profile |Ez/E0|2 for an ultra-short and tightly-focused Bessel pulse of order l = 2, at the instants (following generation at t = 0) of t = 10 fs, 10 ps and 1 ns. (a–c) display behavior during propagation in vacuum and (e–g) in an under-dense plasma of ambient electron density n0 = 1020 cm−3. From both sets of figures, one sees that the pulse propagates without distortion, neither by dispersion nor by diffraction. Over the time interval from 0 to 1 ns, the centroid of the pulse covers a distance, in the propagation direction, of about 30 cm, with the pulse-shape remaining almost intact. (d) and (h) show variations with the radial distance r of the axial intensity profile in the plane z = ct. Comparison of (d) with (h) reveals that the presence of a plasma background alters the central intensity maximum by roughly 10%, compared to its vacuum-based counterpart, for the parameter set used. For this particular set of parameters, the fields are enhanced by the presence of the plasma.
Discussion
Fields of an ultra-short and tightly-focused Bessel pulse of arbitrary order have been derived. The expressions presented and discussed in this paper are fully analytic, but approximate. They have been arrived at strictly analytically from a one-component vector potential polarized along the propagation direction of the pulse, together with a scalar potential linked to the said vector potential by the Lorentz gauge. Vector potential of the pulse of finite extension has been synthesized, like a wavepacket, from Fourier components of a uniform wavenumber distribution. The full vector potential has been given as a power-series expansion and the leading (zeroth-order) term only has been used to derive the electric and magnetic field components reported in this paper. Intensity profiles of the field components have been discussed and shown to propagate like those of a laser bullet, without distortion by dispersion or diffraction. Because of the presence of two Bessel functions in the expression giving the zeroth-order vector potential, the pulse deserved the designation as a “Bessel-Bessel laser bullet”.
As the figures presented above show, fields of the orbital-angular-momentum-carrying Bessel-Bessel bullets have complicated intensity distributions, with some of them possessing sizable background radial oscillations, in addition to the main/central peaks. To rid a typical pulse of its background oscillations and make it useful for such applications as laser-acceleration, considerable pre- and post-pulse work may be required, which can alter the intensity and impact the efficacy of the process in question. Furthermore, in applications like HHG, the polarization and carrier envelope phase of the pulse play important roles. Control of the polarization-related effects and CEP stability may turn out to be challenging for the laser technology that would aim for experimental realization and ultimate utilization of a Bessel-Bessel bullet.
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The author thanks C. H. Keitel for fruitful discussions and a critical reading of the manuscript.
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Salamin, Y.I. Fields of a Bessel-Bessel light bullet of arbitrary order in an under-dense plasma. Sci Rep 8, 11362 (2018). https://doi.org/10.1038/s41598-018-29694-y
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DOI: https://doi.org/10.1038/s41598-018-29694-y
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