Skip to main content
Log in

240Pu/239Pu atom ratios in the bottom sediments of the NW Pacific Ocean

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

239+240Pu concentrations and 240Pu/239Pu atom ratios in bottom sediments of the Yellow Sea, Korea Strait, East Sea (Sea of Japan), Sea of Okhotsk, and Northwest Pacific Ocean were determined. In coastal sediments near the Korean Peninsula, 239+240Pu concentrations varied from 0.02 to 1.72 Bq.kg-1, and their 240Pu/239Pu atom ratios from 0.15 to 0.24, with an average of 0.20±0.03. 240Pu/239Pu atom ratios of bottom sediments in the deep NW Pacific Ocean and its marginal seas (East, Okhotsk seas) were in the range of 0.15-0.23. A little elevated 240Pu/239Pu atom ratios in the bottom layer sediment may be due to Pu released into the environment during the pre-moratorium period, having high 240Pu/239Pu atom ratios and low 238Pu/239+240Pu activity ratios.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Similar content being viewed by others

References

  1. A. V. Yablokov, V. K. Karasev, V. M. Rumyantsev et al., White Book: Facts and Problems Related to Radioactive Waste Disposal in Seas Adjacent to the Territory of the Russian Federation, Office of the President of the Russian Federation, Moscow, 1993.

    Google Scholar 

  2. Investigation of Environmental Radioactivity in Waste Dumping Areas in the Northwest Pacific Ocean: Results of the Second Stage Japanese-Korean-Russian Joint Expedition, Report 1995, Science and Technology Agency, Tokyo, 1997, p. 1.

  3. H. B. L. Petterson, H. Amano, V. I. Berezhnov et al., Sci. Total Environ., 237/238 (1999) 213.

    Google Scholar 

  4. K. Hirose, H. Amano, M. S. Baxter et al., J. Environ. Radioact., 43 (1999) 1.

    Google Scholar 

  5. Y. Ikeuchi, H. Amano, M. Aoyama et al., Sci. Total Environ., 237/238 (1999) 203.

    Google Scholar 

  6. K. O. Buesseler, J. Environ. Radioact., 36 (1997) 69.

    Google Scholar 

  7. L. W. Cooper, J. M. Kelley, L. A. Bond, K. A. Orlandin, J. M. Grebmeier, Marine Chemistry, 69 (2000) 253.

    Google Scholar 

  8. C. K. Kim, C. S. Kim, B. U. Chang, C. S. Chung, G. H. Hong, K. Hirose, Y. Igarashi, Sci. Total Environ., to be published.

  9. C. S. Kim, C. K. Kim, J. I. Lee, K. J. Lee, J. Anal. At. Spectrom., 15 (2000) 247.

    Google Scholar 

  10. M. Koide, K. K. Bertine, T. J. Chow, Earth Planet. Sci. Lett., 72 (1985) 1.

    Google Scholar 

  11. P. W. Krey, E. P. Hardy, C. Pachucky, F. Rourke, J. Coluzza, W. K. Benson, Mass Isotopic Composition of Global Fallout Pu in Soils. Transuranium Nuclides in the Environment, IAEA-SM-199/39, IAEA, Vienna, 1976, p. 671.

    Google Scholar 

  12. G. H. Hong, S. H. Kim, C. S. Chung, D. J. Kang, D. H. Shin, H. J. Lee, S. J. Han, Geo-Marine Letters, 17 (1997) 126.

    Google Scholar 

  13. J. K. Cochran, Geochim. Cosmochim. Acta, 49 (1985) 1195.

    Google Scholar 

  14. Y. Nagaya, K. Nakamura, Distributions and Mass-Balance of 239.240Pu and 137Cs in the Northern North Pacific. Deep Ocean Circulation, Physical and Chemical Aspects, T. Teramoto (Ed.), Elsevier Science Publishers, 1993, p. 157.

  15. H. D. Livingston, P. P. Povinec, T. Ito, O, Togawa, The Behaviour of Plutonium in the Pacific Ocean, in: Plutonium in the Environment, A. Kudo (Ed.), Elsevier Science Ltd., 2001, p. 267.

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Kim, C.K., Kim, C.S., Chang, B.U. et al. 240Pu/239Pu atom ratios in the bottom sediments of the NW Pacific Ocean. Journal of Radioanalytical and Nuclear Chemistry 258, 265–268 (2003). https://doi.org/10.1023/A:1026225402410

Download citation

  • Issue Date:

  • DOI: https://doi.org/10.1023/A:1026225402410

Keywords

Navigation