Hostname: page-component-8448b6f56d-m8qmq Total loading time: 0 Render date: 2024-04-24T16:35:09.424Z Has data issue: false hasContentIssue false

14C Levels in the Vicinity of Two Swedish Nuclear Power Plants and at Two “Clean-Air” Sites in Southernmost Sweden

Published online by Cambridge University Press:  18 July 2016

Kristina Stenström
Affiliation:
Department of Nuclear Physics, Lund University, Sölvegatan 14, SE-223 62 Lund, Sweden
Göran Skog
Affiliation:
Radiocarbon Dating Laboratory, Department of Quaternary Geology, Lund University, Tornavägen 13, SE-223 62 Lund, Sweden
Charlotte Thornberg
Affiliation:
Department of Radiation Physics, Lund University, Malmö University Hospital, SE-205 02 Malmö, Sweden
Bengt Erlandsson
Affiliation:
Department of Nuclear Physics, Lund University, Sölvegatan 14, SE-223 62 Lund, Sweden
Ragnar Hellborg
Affiliation:
Department of Nuclear Physics, Lund University, Sölvegatan 14, SE-223 62 Lund, Sweden
Sören Mattsson
Affiliation:
Department of Radiation Physics, Lund University, Malmö University Hospital, SE-205 02 Malmö, Sweden
Per Persson
Affiliation:
Department of Nuclear Physics, Lund University, Sölvegatan 14, SE-223 62 Lund, Sweden
Rights & Permissions [Opens in a new window]

Abstract

Core share and HTML view are not available for this content. However, as you have access to this content, a full PDF is available via the ‘Save PDF’ action button.

14C is one of the radionuclides that are produced to different degrees by neutron-induced reactions in all types of nuclear reactors. Part of the 14C created is continuously released into the surrounding environment during normal operation as airborne effluents in various chemical forms (such as CO2, CO and hydrocarbons) through the ventilation system of the plant. Because of the biological importance of carbon and the long half-life of 14C, it is of interest to measure the releases and their incorporation into living material. We report here on the 14C activity concentrations in annual tree rings and the air around two Swedish nuclear power plants, as well as the background 14C activity levels from two reference sites in southern Sweden from 1973–1996. We used both accelerator mass spectrometry (AMS) and decay counting in the investigation.

Type
Part 1: Methods
Copyright
Copyright © The American Journal of Science 

References

Burchuladze, A. A., Chudy, M., Eristavi, I. V., Pagava, S. V., Povinec, P., Sivo, A. and Togonidze, G. I. 1989 Anthropogenic 14C variations in atmospheric CO2 and wines. In Long, A., Kra, R. S. and Srdoč, D., eds., Proceedings of the 13th International 14C Conference. Radiocarbon 31(3): 771776.CrossRefGoogle Scholar
Donahue, D. J., Linick, T. W. and Jull, A. J. T. 1990 Isotope-ratio and background corrections for accelerator mass spectrometry radiocarbon measurements. Radiocarbon 32(2): 135142.Google Scholar
Håkansson, S. 1968 University of Lund Radiocarbon dates I. Radiocarbon 10: 3654.CrossRefGoogle Scholar
Håkansson, S. 1977 University of Lund Radiocarbon dates X. Radiocarbon 19(3): 424441.Google Scholar
Håkansson, S. 1986 University of Lund Radiocarbon dates XIX. Radiocarbon 28(3): 11111152.Google Scholar
Håkansson, S. 1987 University of Lund Radiocarbon dates XX. Radiocarbon 29(3): 353379.Google Scholar
Håkansson, S. 1988 University of Lund Radiocarbon dates XXI. Radiocarbon 30(2): 179196.Google Scholar
Håkansson, K., Hellborg, R., Erlandsson, B., Skog, G., Stenström, K. and Wiebert, A. 1996 A cesium-sputtering negative ion source for AMS investigations. Nuclear Instruments and Methods in Physics Research A382: 327331.Google Scholar
Hertelendi, E., Uchrin, G. and Ormai, P. 1989 14C release in various chemical forms with gaseous effluents from the Paks Nuclear Power Plant. In Long, A., Kra, R. S. and Srdoč, D., eds., Proceedings of the 13th International 14C Conference. Radiocarbon 31(3): 754761.Google Scholar
Kunz, C. 1985 Carbon-14 discharge at three light-water reactors. Health Physics 49(1): 2535.Google Scholar
Levin, I. and Kromer, B. 1997 Twenty years of high-precision atmospheric 14CO2 observations at Schauinsland station, Germany. Radiocarbon 39(2): 205218.Google Scholar
Levin, I., Kromer, B., Barabas, M. and Münnich, K. O. 1988 Environmental distribution and long-term dispersion of reactor 14CO2 around two German nuclear power plants. Health Physics 54(2): 149156.Google Scholar
Levin, I., Kromer, B., Schoch-Fischer, H., Bruns, M., Münnich, M., Berdau, D., Vogel, J. C. and Münnich, K.O. 1985 25 years of tropospheric 14C observations in central Europe. Radiocarbon 27(1): 119.CrossRefGoogle Scholar
Levin, I., Schuchard, J., Kromer, B. and Münnich, K. O. 1989 The continental European Suess effect. In Long, A., Kra, R. S. and Srdoč, D., eds., Proceedings of the 13th International 14C Conference. Radiocarbon 31(3): 431440.CrossRefGoogle Scholar
Olsson, I. U. 1989 Recent 14C activity in the atmosphere, “clean air” and the Chernobyl effect. In Long, A., Kra, R. S. and Srdoč, D., eds., Proceedings of the 13th International 14C Conference. Radiocarbon 31(3): 740746.CrossRefGoogle Scholar
Meijer, H. A. J., van der Plicht, H., Gislefoss, J. S. and Nydal, R. 1994 Comparing long-term atmospheric 14C and 3H records near Groningen, the Netherlands with Fruholmen, Norway and Izaña, Canary Islands 14C stations. Radiocarbon 37(1): 3950.Google Scholar
Olsson, I. U. and Possnert, G. 1992 14C activity in different sections and chemical fractions of oak tree rings, AD 1938–1981. In Long, A. and Kra, R. S., eds., Proceedings of the 14th International 14C Conference. Radiocarbon 34(3): 757767.Google Scholar
Otlet, R. L., Walker, A. J., Fulker, M. J. and Collins, C. 1997 Background carbon-14 levels in UK foodstuffs, 1981–1995, based upon a 1992 survey. Journal of Environmental Radioactivity 34(1): 91101.Google Scholar
Snellman, M. 1988 Sampling and monitoring of carbon-14 in gaseous effluents from nuclear facilities—A literature survey. Project SSI P 498.88.Google Scholar
Stenström, K. 1995 New Applications of 14 C Measurements at the Lund AMS Facility . Doctoral Dissertation, Lund University, ISBN 91-628-1816-3: 167 p.Google Scholar
Stenström, K., Erlandsson, B., Hellborg, R., Skog, G. and Wiebert, A. 1996a Determination of the 14CO2 and total airborne 14C releases from two Swedish light-water reactors using accelerator mass spectrometry. Radioactivity and Radiochemistry 7(1): 3236.Google Scholar
Stenström, K., Erlandsson, B., Hellborg, R., Wiebert, A. and Skog, G. 1996b Environmental levels of carbon-14 around a Swedish nuclear power plants measured with accelerator mass spectrometry. Nuclear Instruments and Methods in Physics Research B113: 474476.Google Scholar
Stenström, K., Erlandsson, B., Hellborg, R., Wiebert, A., Skog, G., Vesanen, R., Alpsten, M. and Bjurman, B. 1995 A one-year study of the total air-borne 14C effluents from two Swedish light-water reactors, one boiling water- and one pressurized water reactor. Journal of Radioanalytical and Nuclear Chemistry 198(1): 203213.Google Scholar
Stenström, K., Leide-Svegborn, S., Erlandsson, B., Hellborg, R., Skog, G., Mattsson, S., Nilsson, L.-E., and Nosslin, B. 1997 A programme for long-term retention studies of 14C-labelled compounds in man using the Lund AMS facility. Nuclear Instruments and Methods in Physics Research B123: 245248.CrossRefGoogle Scholar
Stuiver, M. and Polach, H. A. 1977 Discussion: Reporting of 14C data. Radiocarbon 19(3): 355363.Google Scholar
Uchrin, G., Csaba, E., Hertelendi, E., Ormai, P. and Barnabas, I. 1992 14C release from a Soviet-designed pressurized water reactor nuclear power plant. Health Physics 63(6): 651655.Google Scholar
UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) 1988 Effects and Risks of Ionizing Radiation. New York, United Nations. Annex B: 159161.Google Scholar
Vogel, J. S., Southon, J. R., Nelson, D. E. and Brown, T. A. 1984 Performance of catalytically condensed carbon for use in accelerator mass spectrometry. Nuclear Instruments and Methods in Physics Research B5: 289293.Google Scholar
Wahlen, M. and Kunz, C.O. 1978a 14C discharge from boiling water reactors. Trans. American Nuclear Society 28: 7475.Google Scholar
Wahlen, M. and Kunz, C.O. 1978b 14C activity and distribution in gaseous effluents from pressurized water reactors. Transactions of the American Nuclear Society 30: 113114.Google Scholar
Wiebert, A. 1995 Development of the Lund AMS Facility and the Evaluation of a New AMS Detection Technique. Doctoral Dissertation, University of Lund, ISBN 91-628-1713-2: 96 p.Google Scholar
Winkelmann, I. and Vogl, K. 1984 Measurement of specific radionuclides in gaseous effluents from nuclear power plants and their contribution to radiation exposure. In Kaul, A., Neider, R., Pensko, J., Stieve, F.-E. and Brunner, H., eds., Radiation - Risk - Protection . Rheinland, Verlag TÜV: 875878.Google Scholar