Large-scale radon hazard evaluation in the Oslofjord region of Norway utilizing indoor radon concentrations, airborne gamma ray spectrometry and geological mapping
Introduction
Radon gas is the largest natural source of human exposure to ionising radiation and most of that exposure occurs at home (UNSCEAR, 2000). Recent studies in Europe (Darby et al., 2005, Darby et al., 2006), North America (Krewski et al., 2005, Krewski et al., 2006) and China (Lubin et al., 2004) present overwhelming evidence in support of the traditionally held view that prolonged exposure to radon is responsible for many new cases of lung cancer each year, and offer estimates of the magnitude of the risk. The European study revealed a statistically significant relationship between levels of exposure to radon and the incidence of lung cancer that persists down to radon concentrations of 200 Bq m− 3 or lower — the radon action level in most countries. This verifies studies based on cancer cases among miners exposed to radon and its progenies at work (BEIR VI, 1999) and further suggests that long term exposure to radon represents a risk to health even at low concentrations.
Although there are several epidemiological studies of possible relationships between radon and other forms of cancer such as leukaemia (Raaschou-Nielsen et al., 2008), and between radon and other diseases like multiple sclerosis (Bølviken et al., 2003), the analyses have not been able to demonstrate any clear associations between the diseases and radon. Therefore it is probable that lung cancer represents by far the most significant risk to human health associated with exposure to radon.
Norway has some of the highest concentrations of radon in indoor air in the world. Extensive mapping of radon in indoor air suggests that approximately 175,000 dwellings in Norway, 9% of the total number, have annual average radon concentrations above the action level of 200 Bq m− 3 (Strand et al., 1991, Strand et al., 1992, Strand et al., 2001, Strand et al., 2003). It is further estimated that around 27,000 Norwegians live in dwellings with average radon concentrations above 1000 Bq m− 3 (Lunder Jensen et al., 2004). In the studied area around the capital city of Oslo and Oslofjord (Fig. 1), where approximately half of the Norwegian population live, radon concentrations in dwellings can exceed 5000 Bq m− 3 (Strand et al., 2001, Strand et al., 2003).
The substrate beneath dwellings is the principal source of radon in Norwegian homes (Stranden, 1986). The amount of radium in the ground determines the amount of radon generated there. The concentration of radium in different rock types varies from under 10 Bq kg− 1 in sandstone and limestone to several thousand Bq kg− 1 in alum shale (Andersson et al., 1985, Nordic, 2000). Radon is a special problem in the investigated area because alum shale and soils derived from it occur in well populated areas (Stranden and Strand, 1988). Also, much of this most densely populated part of Norway is underlain by the Oslo Rift, containing large volumes of radium bearing magmatic rocks (Ramberg and Larsen, 1978, Ro et al., 1990, Neumann et al., 2004). Adding to the hazard profile of the region, large bodies of radium rich granitic gneiss occur in populated areas outside the rift (Slagstad, 2006, Bingen et al., 2008).
Transport of radon in pore spaces in the ground up to a building is through convection or diffusion depending on factors such as water content and permeability of the ground (Tanner, 1964, Nero and Nazaroff, 1984, Nazaroff, 1992). In low permeability materials such as marine silt and clay, occurring locally in the investigated area, radon emanation can reach 70% but transport of radon is minimal so these materials are generally associated with a low radon hazard level. Emanation is lower in glacio-fluvial sand and gravel deposits, common in the investigated area, but their higher permeability permits the transport of much more of the emanated fraction of radon towards a building's foundations (Stranden et al., 1985, Åkerblom et al., 1990, Peake, 1988, Hutri and Mäkeläinen, 1993, Sundal et al., 2004a). Therefore glacio-fluvial deposits make a significant contribution to the radon hazard profile of the investigated area.
Programmes for the mapping of radon in the housing stock of the Oslo/Oslofjord region have been orchestrated by the Norwegian Radiation Protection Authority over many years as most recently documented by Strand et al., 1991, Strand et al., 1992, Strand et al., 2001, Strand et al., 2003. The programmes are largely founded on measurements of radon concentrations in indoor air in homes selected at random from the housing stock. However, given the strong spatial variability in geological conditions governing radon emanation and transport in the region, geologically focused investigations have also been carried out (e.g. Stranden and Strand, 1986, Stranden and Strand, 1988, Sundal et al., 2004b).
In 2004 the Norwegian Radiation Protection Authority joined forces with the Geological Survey of Norway to examine new ways to combine available geological data with indoor radon measurements to establish a new overview of spatially variable radon hazard levels across the Oslo/Oslofjord region. That initiative comprised the construction of a geographic information system containing information on radon measurements in the housing stock, bedrock geology, drift geology (superficial deposits) and airborne gamma ray spectrometer data. The data sets were analyzed and their implications for radon hazard combined into radon awareness maps with an accompanying explanation (Smethurst et al., 2006 [in Norwegian]; maps available from http://www.ngu.no).
The present contribution presents the findings of that cross-institution initiative. We go further than that investigation by taking the hazard indications from the individual data sets and compounding them into a single radon awareness map theme layer that records awareness level (high or moderate) and which data types triggered the assignment of elevated hazard. This theme is currently being made available to Norwegian planning authorities through the national AREALIS interactive map service co-ordinated by the Norwegian Mapping Authority (http://www.ngu.no/kart/arealis [in Norwegian]).
Section snippets
Radon in indoor air
Around 80,000 radon measurements have been made in Norwegian dwellings (4.2% of the housing stock); approximately 55,000 of these by the Norwegian Radiation Protection Authority (NRPA; Strand et al., 2001, Strand et al., 2003). The measurements were made using alpha-track detectors placed in living- and bedrooms, integrating over at least two months, usually in the winter. The NRPA have converted these to estimates of annual average radon concentration using a simple model for seasonal
Using uranium concentrations from airborne gamma ray spectrometry to predict radon hazard
We and many others before us have observed that uranium maps from airborne gamma ray spectrometer surveys can provide valuable first-order information on the distribution of elevated radon concentrations in dwellings (e.g. Doyle et al., 1990, Duval and Otton, 1990, Åkerblom, 1995). Exactly how useful the airborne data may be depends on the specifications of the surveys, ground conditions, climate, styles of dwelling construction and methods of heating and ventilating dwellings. Here we start
Superposing different radon hazard criteria to produce a single hazard forecast
It is clear that as long as indoor radon concentration measurements are few in number or restricted in geographic spread, and there is interest in potential radon hazards in previously unsettled terrain, information on potential radon hazards must be drawn from other datasets. We have shown that bedrock and drift geology provide important information in the evaluation of radon hazard, and we have also demonstrated that airborne geophysical measurements can be used to identify large areas that
Conclusions
We compiled geological data relevant to radon hazard in dwellings in the Oslo region of Norway and generated region-wide radon hazard maps. In particular we tested the usefulness of airborne gamma ray spectrometer surveying as a method of locating areas with elevated radon hazard levels.
We found a simple linear relationship between uranium concentration in the ground from airborne surveying and the proportion of dwellings with average annual radon concentrations above the action level of 200 Bq
Acknowledgements
This work was carried out as part of the Geological Survey of Norway's geology for society in the Oslo region programme in co-operation with the Norwegian Radiation Protection Authority. Arne Bjørlykke of the Survey and Ole Harbitz of NRPA were integral in establishing the co-operation. Our thanks go to John Dehls, Tor Erik Finne, Bernard Bingen and Bjørn Bergstrøm of the Geological Survey of Norway for their assistance in building the GIS.
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At the Norwegian Radiation Protection Authority while participating in the research presented here.