Constraints on the acquisition of remanent magnetization in fine-grained sediments imposed by redeposition experiments
Introduction
For some 50 yr, the remanent magnetization of sediments has been widely used in a large variety of applications. These studies have improved our knowledge of the earth's magnetic field over time scales covering almost the entire range of field variability (from hundreds to millions of years). The data have also been applied to problems concerning tectonic deformation, crustal block rotations and environmental studies. More broadly, these data provide important constraints on the geodynamics of the deep earth and are important to problems ranging from the growth of the inner core to mantle convection. Paleomagnetic constraints on these problems are unique in comparison with others in that they can resolve these problems in terms of geological history.
Considering the importance of sedimentary paleomagnetic records, our understanding of the physical processes that control detrital remanent magnetization (DRM) is woefully underdeveloped. (For the sake of clarity, we define DRM as a magnetization produced by settling or the physical agitation of the sediment and post-depositional remanent magnetization [pDRM] as a magnetization produced in settled sediments by a field [H] of similar magnitude to the earth's by magnetic grains that are free to mechanically rotate parallel to H without physical agitation of the sediment.) As we pursue increasingly detailed paleomagnetic records, it becomes critical to understand how these records filter the signal of the earth's magnetic field. The problem is a simple convolution, m = f ⁎ s, where m is the paleomagnetic record, s is the true variation of the earth's magnetic field and f is the filter, or transfer function that controls any lag or smoothing that may be present in the imperfect recording of the field.
The most recent published redeposition experiments were conducted by Katari et al. [1] who concluded that f causes no smoothing of s and that, at most, causes an unspecified amount of lag. Their conclusion is uncertain because they did observe evidence for smoothing, but claimed that it was due to a thermally activated viscous remanent magnetization (VRM). In spite of this claim, Katari et al. [1] could not completely rule out the possibility that they had observed a true pDRM. The existence of pDRM has been defended in previous laboratory experiments [2], [3], [4], [5], [6] and also on the basis of paleomagnetic observations from sediment cores [7]. Katari et al. [1] pointed out that the observed pDRM involved samples that were dried in order to produce a consolidated sample. They then argued that the drying out process could be an important factor in producing the pDRM. For most sediments, drying does not play a role in consolidation and, thus, these experiments may not be applicable. In summary, one cannot say whether or not pDRM smoothes s based on previous laboratory experiments.
Technical difficulties involved in simulating DRM in the laboratory have substantially hindered the development of our understanding of DRM. Simple gravitational settling of fine-grained material is often not sufficient to consolidate the sediment [8] and fine sediment can stabilize at high water concentrations. The sediments used in the present experiments stabilize at ∼ 80% water by mass (all percents given are mass based). Two techniques have previously been employed to address this major difficulty. Both approaches generate critical problems. Some experimentalists [5], [9], [10] removed water through drying and/or filtering but drying might disturb the fabric of sediment and produce a “drying remanence”. Others [1], [11], [12], [13] used a cryogenic magnetometer to measure unconsolidated sediment without disturbing its fragile fabric. However, such measurements have been made in zero field; therefore magnetic grains that are not “locked in” can rotate away from their magnetized position when removed from the field in which the deposition took place. Grains that would contribute to a pDRM would be in such a state. Measurements performed on unconsolidated sediments are, thus, particularly maladapted to detect pDRM.
Section snippets
Experimental technique
In order to overcome the difficulties discussed above, we performed redeposition experiments using a dilute solution of gelatin (5%). Gelatin is a biopolymer that when present in an aqueous solution gels at temperatures below ∼20 °C. The gelation is caused by the association of polymer chains through non-covalent junction zones [14]. Above the gelation temperature (Tg), the polymers are in a “coiled state”. A 5% solution of gelatin is a Newtonian fluid with a similar dynamic viscosity, ∼ 0.003
Testing DRM versus VRM: DRM as a function of time in zero-field
The first experiment was designed to test the necessity of using gelatin in redeposition experiments. Two samples of Site-851 sediment were prepared with c ∼ 20% by stopping at step 5, as described in Section 2.1. For one sample, gelatin was added to a concentration of 5%, following steps 6–7 in Section 2.1. None was added to the second so as to furnish a control sample. While at 50 °C the sample with gelatin was placed in a vertical 50 μT field, was manually stirred with a small spatula (stirring
Measuring the pDRM at Site 851
The data shown in Fig. 1 lead to the critical conclusion that a stabilized sediment slurry, which is no longer settling, can contain a large percentage of magnetic grains that are free to align with an applied magnetic field at the time of deposition as well as free to mechanically disorient when removed from a magnetic field. Moreover, the time scale of this process is rapid. To complicate matters, the magnetization that remains appears to be stable on much longer time scales. This must be
Conclusions
So far, most attempts to simulate the acquisition of magnetization using redeposition of sediments in the laboratory lacked a direct comparison with the natural remanent magnetization. Through the use of a new experimental technique and by comparing our laboratory data with the NRMs found in the sediment, we observed the following:
- (1)
Sediment that has ceased settling under gravity contains mechanically mobile grains that mechanically disorient when placed in a zero field and that may be
Acknowledgements
This study was partly supported by the French INSU-CNRS program Dynamique et Evolution de la Terre interne. During the final stages of this work B. Carter-Stiglitz was supported by grant 0218384 from the Instruments and Facilities Program, National Science Foundation. We thank A. Roberts and L. Tauxe for helpful reviews; we further thank L. Tauxe for numerous invaluable discussions concerning this work.
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