Skip to main content
SpringerLink
Log in

Microwave Dielectric Properties of Na5RE(MoO4)4 (RE = La, Gd, Dy, Er) Ceramics with a Low Sintering Temperature

  • Published:
Journal of Electronic Materials Aims and scope Submit manuscript

Abstract

Na5RE(MoO4)4 (RE = La, Gd, Dy, Er) ceramics have been synthesized by the conventional solid-state reaction method. The crystallizations, microstructures and microwave dielectric properties of Na5RE(MoO4)4 ceramics were also investigated. The room-temperature x-ray diffraction patterns of Na5RE (MoO4)4 ceramics illustrate a tetragonal structure with a I 41/a space group. The grain size of Na5La(MoO4)4 is larger than that of Na5RE(MoO4)4 (RE = Gd, Dy, Er) ceramics, and uneven grains are observed in the systems. Na5RE (MoO4)4 ceramics sintered at 570–690°C for 4 h possess excellent microwave dielectric properties with εr = 6.4–8.4, τf = − 27.7–34.3 ppm/°C, and Q × f = 4073–24411 GHz at their optimum sintering temperature. The nonreactivity of Na5Er(MoO4)4 with silver is evidenced by x-ray diffraction, and SEM and EDS analysis reveal that silver can be a co-firable electrode material for the present ceramics.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Log in via an institution

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Similar content being viewed by others

References

  1. L. Fang, D. Chu, H. Zhou, X. Chen, H. Zhang, B. Chang, C. Li, Y. Qin, and X. Huang, J. Alloys Compd. 509, 8840 (2011).

    Article  Google Scholar 

  2. H. Yang, Y. Lin, J. Zhu, F. Wang, and Z. Dai, J. Alloys Compd. 502, L20 (2010).

    Article  Google Scholar 

  3. R. Umemura, H. Ogawa, and A. Kan, J. Eur. Ceram. Soc. 26, 2063 (2006).

    Article  Google Scholar 

  4. S. Kawashima, M. Nishida, I. Ueda, and H. Ouchi, J. Am. Ceram. Soc. 66, 421 (1983).

    Article  Google Scholar 

  5. K.P. Surendran, N. Santha, P. Mohanan, and M.T. Sebastian, Eur. Phys. J. B 41, 301 (2004).

    Article  Google Scholar 

  6. A. Belous, O. Ovchar, D. Durilin, M.M. Krzmanc, M. Valant, and D. Suvorov, J. Am. Ceram. Soc. 89, 3441 (2006).

    Article  Google Scholar 

  7. W. Lei, W.Z. Lu, D. Liu, and J.H. Zhu, J. Am. Ceram. Soc. 92, 105 (2009).

    Article  Google Scholar 

  8. Y.I. Sohn, J. Inaguma, S.O. Yoon, M. Itoh, T. Nakamura, S.J. Yoon, and H.J. Kim, Jpn. J. Appl. Phys. 33, 5466 (1994).

    Article  Google Scholar 

  9. X. Chou, J. Zhai, and X. Yao, Appl. Phys. Lett. 91, 122908 (2007).

    Article  Google Scholar 

  10. M.M. Mao, X.C. Fan, and X.M. Chen, Int. J. Appl. Ceram. Technol. 7, E156 (2010).

    Article  Google Scholar 

  11. D. Zhou, L.X. Pang, J. Guo, G.Q. Zhang, Y. Wu, H. Wang, and X. Yao, J. Eur. Ceram. Soc. 31, 2749 (2011).

    Article  Google Scholar 

  12. J. Dhanya, A.V. Basiluddeen, and R. Ratheesh, Scr. Mater. 132, 1 (2017).

    Article  Google Scholar 

  13. L.X. Pang, H. Liu, D. Zhou, G.B. Sun, W.-G. Qin, and W.G. Liu, Mater. Lett. 72, 128 (2012).

    Article  Google Scholar 

  14. V.A. Morozov, B.I. Lazoryak, S.Z. Shmurak, A.P. Kiselev, O.I. Lebedev, N. Gauquelin, J. Verbeeck, J. Hadermann, and G. Van Tendeloo, Chem. Mater. 26, 3238 (2014).

    Article  Google Scholar 

  15. D. Zhou, C.A. Randall, L.-X. Pang, H. Wang, J. Guo, G.-Q. Zhang, Y. Wu, K.-T. Guo, L. Shui, and X. Yao, Mater. Chem. Phys. 129, 688 (2011).

    Article  Google Scholar 

  16. Z. Wang, C. Yuan, Q. Li, Q. Feng, F. Liu, C. Zhou, G. Chen, and G. Rao, J. Mater. Sci. Mater. Electron. 28, 9941 (2017).

    Article  Google Scholar 

  17. C. Guo, F. Gao, Y. Xu, L. Liang, F.G. Shi, and B. Yan, J. Phys. D Appl. Phys. 42, 095407 (2009).

    Article  Google Scholar 

  18. J. Dhanya, E. Kalathil Suresh, R. Naveenraj, and R. Ratheesh, Ceram. Int. 44, 6699 (2018).

    Article  Google Scholar 

  19. S. Parida, S.K. Rout, L.S. Cavalcante, E. Sinha, M.S. Li, V. Subramanian, N. Gupta, V.R. Gupta, J.A. Varela, and E. Longo, Ceram. Int. 38, 2129 (2012).

    Article  Google Scholar 

  20. D. Zhou, C.A. Randall, L.X. Pang, H. Wang, J. Guo, G.Q. Zhang, X.G. Wu, L. Shui, and X. Yao, J. Am. Ceram. Soc. 94, 348 (2011).

    Article  Google Scholar 

  21. L.X. Pang, G.B. Sun, and D. Zhou, Mater. Lett. 65, 164 (2011).

    Article  Google Scholar 

  22. K.H. Yoon, W.S. Kim, and E.S. Kim, Mater. Sci. Eng. B 99, 112 (2003).

    Article  Google Scholar 

Download references

Acknowledgments

The authors would like to thank the National Natural Science Foundation of China (Grant No. 11464006) for financial support.

Author information

Authors and Affiliations

  1. College of Material Science and Engineering, Guilin University of Electronic Technology, Guilin, 541004, People’s Republic of China

    Liufang Meng, Changlai Yuan, Baohua Zhu, Xiao Liu, Fei Liu, Jiwen Xu, Changrong Zhou & Guohua Chen

  2. Guangxi Key Laboratory of Information Materials, Guilin University of Electronic Technology, Guilin, 541004, People’s Republic of China

    Changlai Yuan, Xiao Liu, Jiwen Xu, Changrong Zhou & Guohua Chen

Authors
  1. Liufang Meng
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. Changlai Yuan
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. Baohua Zhu
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. Xiao Liu
    View author publications

    You can also search for this author in PubMed Google Scholar

  5. Fei Liu
    View author publications

    You can also search for this author in PubMed Google Scholar

  6. Jiwen Xu
    View author publications

    You can also search for this author in PubMed Google Scholar

  7. Changrong Zhou
    View author publications

    You can also search for this author in PubMed Google Scholar

  8. Guohua Chen
    View author publications

    You can also search for this author in PubMed Google Scholar

Corresponding author

Correspondence to Changlai Yuan.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Meng, L., Yuan, C., Zhu, B. et al. Microwave Dielectric Properties of Na5RE(MoO4)4 (RE = La, Gd, Dy, Er) Ceramics with a Low Sintering Temperature. J. Electron. Mater. 48, 656–661 (2019). https://doi.org/10.1007/s11664-018-6775-7

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11664-018-6775-7

Keywords

Search

Navigation