Skip to main content

Advertisement

Log in

Evaluation of natural radioactivity levels and potential radiological hazards of common building materials utilized in Mediterranean region, Turkey

  • Research Article
  • Published:
Environmental Science and Pollution Research Aims and scope Submit manuscript

Abstract

Radiometric measurement of building materials is very important to assess the internal and external exposure caused by the ionizing radiation emitted from terrestrial radionuclides in building materials. The activity concentrations of 226Ra, 232Th, and 40K in fifty-eight samples of fifteen different structural and covering building materials commonly used in Osmaniye province located in the Mediterranean region of Turkey were measured by using gamma-ray spectroscopy. The activity concentrations of 226Ra, 232Th, and 40K varied from 2.5 ± 0.1 (marble) to 145.7 ± 4.4 (clay brick), 1.3 ± 0.1 (marble) to 154.3 ± 4.1 (marble), and 8.6 ± 0.2 (sand) to 1044.1 ± 70.3 (granite), respectively. Radiological parameters (activity concentration index, alpha index, indoor absorbed gamma dose rate and the corresponding annual effective dose rate, and excess lifetime cancer risk) were estimated to evaluate the health hazards associated with these building materials. Since the estimated values of these parameters are within the recommended safety limits or criteria values, the use of the studied building materials in the construction of dwellings can be considered to be safe for the residents of the region.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2

Similar content being viewed by others

Data availability

All data generated or analyzed during this study are included in this published article; anyway, datasets are available from the corresponding author on reasonable request.

References

  • Abdullahi S, Ismail AZ, Samat S (2019) Determination of indoor doses and excess lifetime cancer risks caused by building materials containing natural radionuclides in Malaysia. Nucl Eng Technol 51:325–336

    CAS  Google Scholar 

  • Aladeniyi K, Arogunjo AM, Pereira AJSC, Khandaker MU, Bradley DA, Sulieman A (2021) Evaluation of radiometric standards of major building materials used in dwellings of South-Western Nigeria. Radiat Phys Chem 178(109021):1–9

    Google Scholar 

  • Al-Hubail J, Al-Azmi D (2018) Radiological assessment of indoor radon concentrations and gamma dose rates in secondary school buildings in Kuwait. Constr Build Mater 183:1–6

    CAS  Google Scholar 

  • Al-Sewaidan HA (2019) Natural radioactivity measurements and dose rate assessment of selected ceramic and cement types used in Riyadh, Saudi Arabia. J King Saud Univ Sci 31:987–992

    Google Scholar 

  • Asaduzzaman K, Mannan F, Khandaker MU, Farook MS, Elkezza A, Amin YM, Sharma S, Kassim HA (2015) Assessment of natural radioactivity levels and potential radiological risks of common building materials used in Bangladeshi dwellings. PLoS One 10(10):1–16

    Google Scholar 

  • Axelsson G, Andersson EM, Barregard L (2015) Lung cancer risk from radon exposure in dwellings in Sweden: how many cases can be prevented if radon levels are lowered? Cancer Causes Control 26(4):541–547

    Google Scholar 

  • Aykamış AŞ, Turhan Ş, Uğur FA, Baykan UN, Kılıç AM (2013) Natural radioactivity, radon exhalation rates and indoor radon concentration of some granite samples used a construction material in Turkey. Radiat Prot Dosim 157:105–111

    Google Scholar 

  • Baykara O, Karatepe S, Doğru M (2012) Assessments of natural radioactivity and radiological hazards in construction materials used in Elazig, Turkey. Radiat Meas 46(1):153–158

    Google Scholar 

  • Damla N, Cevik U, Kobya AI, Celik A, Grieken RV, Kobya Y (2009) Characterization of gas concrete materials used in buildings of Turkey. J Hazard Mater 168(2–3):681–687

    CAS  Google Scholar 

  • Darby SC, Whitley E, Howe GR, Hutchings SJ, Kusiak RA, Lubin JH, Morrison HI, Tirmarche M, Tomásek L, Radford EP, Roscoe RJ, Samet JM, Yao SX (1995) Radon and cancers other than lung cancer in underground miners: a collaborative analysis of 11 studies. J Natl Cancer Inst 87(5):378–384

    CAS  Google Scholar 

  • De With G, Michalik B, Hoffmann B, Döse M (2018) Use of NORM-containing products in construction development of a European harmonised standard to determine the natural radioactivity concentrations in building materials. Constr Build Mater 171:913–918

    Google Scholar 

  • EC (European Commission) (1999) Radiation Protection 112- Radiological protection principles concerning the natural radioactivity of building materials. Directorate- General Environment, Nuclear Safety and Civil Protection

  • Erees FS, Dayanıklı SA, Çam S (2006) Natural radionuclides in the building materials used in Manisa city, Turkey. Indoor Built Environ 15(5):495–498

    CAS  Google Scholar 

  • Ghias S, Satti KH, Khan M, Dilband M, Naseem A, Jabbar A, Kali S, Rehman TU, Nawab J, Aqeel M, Khan MA, Zafar MI (2021) Health risk assessment of radioactive footprints of the urban soils in the residents of Dera Ghazi Khan, Pakistan. Chemosphere 2671(29171):1–14

    Google Scholar 

  • Hatungimana D, Taşköprü C, İçhedef M, Saç MM, Yazıcı Ş, Aghabaglou AM (2020) Determination of radon and natural radioactivity concentration in some building materials used in İzmir, Turkey. J Green Build 15(1):107–118

    Google Scholar 

  • ICRP (1990) Recommendations of the International Commission on Radiological Protection. Vol. 212 No.1-3, publication 60

  • Imani M, Adelikhah M, Shahrokhi A, Azimpour G, Yadollahi A, Kocsis E, Toth-Bodrogi E, Kovács T (2021) Natural radioactivity and radiological risks of common building materials used in Semnan Province dwellings. Iran Environ Sci Pollut Res 28:41492–41503. https://doi.org/10.1007/s11356-021-13469-6

    Article  CAS  Google Scholar 

  • Kocsis E, Tóth-Bodrogi E, Peka A, Adelikhah M, Kovács T (2021) Radiological impact assessment of different building material additives. J Radioanal Nucl Chem. https://doi.org/10.1007/s10967-021-07897-4

  • Kumara PARP, Mahakumara P, Jayalath A, Jayalath CP (2018) Estimating natural radiation exposure from building materials used in Sri Lanka. J Radiat Res Appl Sci 11:350–354

    CAS  Google Scholar 

  • Kurnaz A, Turhan Ş, Hançerlioğulları A, Gören E, Karataşlı M, Altıkulaç A, Erer AM, Metin O (2020) Natural radioactivity, radon emanating power and mass exhalation rate of environmental soil samples from Karabük province, Turkey. Radiochim Acta 108(7):573–579

    CAS  Google Scholar 

  • Kuzmanović P, Todorović N, Petrović LF, Mrđa D, Forkapić S, Nikolov J, Knežević J (2020) Radioactivity of building materials in Serbia and assessment of radiological hazard of gamma radiation and radon exhalation. J Radioanal Nucl Chem 324:1077–1087

    Google Scholar 

  • La Verde G, Raulo A, D’Avino V, Roca V, Pugliese M (2020) Radioactivity content in natural stones used as building materials in Puglia region analysed by high resolution gamma-ray spectroscopy: preliminary results. Constr Build Mater 239(117668):1–6

    Google Scholar 

  • Leonardi F, Bonczyk M, Nuccetelli C, Wysocka M, Michalik B, Ampollini M, Tonnarini S, Rubin J, Niedbalska K, Trevisi R (2018) A study on natural radioactivity and radon exhalation rate in building materials containing norm residues: preliminary results. Constr Build Mater 173:172–179

    CAS  Google Scholar 

  • Lubin JH, Boice JD Jr, Edling C, Hornung RW, Howe GR, Kunz E, Kusiak RA, Morrison HI, Radford EP, Samet JM, Tirmarche M, Woodward A, Yao SX, Pierce DA (1995) Lung cancer in radon-exposed miners and estimation of risk from indoor exposure. J Natl Cancer Inst 87(11):817–827

    CAS  Google Scholar 

  • Nuccetelli C, Leonardi F, Trevisi R (2020) Building material radon emanation and exhalation rate: need of a shared measurement protocol from the European database analysis. J Environ Radioact 225(106438):1–7

    Google Scholar 

  • Mavi B, Akkurt I (2010) Natural radioactivity and radiation hazards in some building materials used in Isparta, Turkey. Radiat Phys Chem 79:933–937

    CAS  Google Scholar 

  • Orosun MM, Usikalu MR, Oyewumi KJ, Achuka JA (2020) Radioactivity levels and transfer factor for granite mining field in Asa, North-central Nigeria. Heliyon 6:1–6

    Google Scholar 

  • Otoo F, Darko EO, Garavaglia M, Giovani C, Pividore P, Andam AB, Amoako JK, Adukpo OK, Inkoom S, Adu S (2018) Public exposure to natural radioactivity and radon exhalation rate in construction materials used within Greater Accra Region of Ghana. Scientific African 1:1–12

    Google Scholar 

  • Pantelić GK, Todorović DJ, Nikolić JD, Rajačić MM, Janković MM, Sarap NB (2015) Measurement of radioactivity in building materials in Serbia. J Radioanal Nucl Chem 303:2517–2522

    Google Scholar 

  • Parmaksız A (2020) Radiological assessment of the bauxite mining in Turkey and estimation of radiation dose contribution of the red mud as a concrete agent of the model room by using RESRAD-BUILD computer code. J Radioanal Nucl Chem 326:1107–1118

    Google Scholar 

  • Ravisankar R, Raghu Y, Chandrasekaran A, Gandhi MS, Vijayagopal P, Venkatraman B (2016) Determination of natural radioactivity and the associated radiation hazards in building materials used in Polur, Tiruvannamalai District,Tamilnadu, India using gamma ray spectrometry with statistical approach. J Geochem Explor 163:41–52

    CAS  Google Scholar 

  • Sas Z, Doherty R, Kovacs T, Soutsos M, Sha W, Schroeyers W (2017) Radiological evaluation of by-products used in construction and alternative applications; Part I. Preparation of a natural radioactivity database. Constr Build Mater 150:227–237

    CAS  Google Scholar 

  • Shahrokhi A, Kovács T (2021) Radiological survey on radon entry path in an underground mine and implementation of an optimized mitigation system. Environ Sci Eur 33(66):1–14

    Google Scholar 

  • Shahrokhi A, Adelikhah M, Chalupnik S, Kocsis E, Toth-Bodrogi E, Kovács T (2020) adioactivity of building materials in Mahallat, Iran – an area exposed to a high level of natural background radiation – attenuation of external radiation doses. Mater Constr 70(340):1–13

    Google Scholar 

  • Shoeib MY, Thabayneh KM (2014) Assessment of natural radiation exposure and radon exhalation rate in various samples of Egyptian building materials. J Radiat Res Appl Sc 7:174–181

    CAS  Google Scholar 

  • Solak S, Turhan Ş, Uğur FA, Gören E, Gezer F, Yeğingil Z, Yeğingil İ (2014) Evaluation of potential exposure risks of natural radioactivity levels emitted from building materials used in Adana, Turkey. Indoor Built Environ 23(4):594–602

    Google Scholar 

  • Sultan DAO, Turhan Ş, Kurnaz A, Hançerlioğulları A, Kamberli AK, Emeksizoğlu B (2020) Investigation of natural radionuclide and essential metal contents of ancient wheat einkorn (Triticum monococcum L.) grown in Turkey. Radiochim Acta 108:999–1007

    CAS  Google Scholar 

  • Stoulos S, Manolopoulou M, Papastefanou C (2003) Assessment of natural radiation exposure and radon exhalation from building materials in Greece. J Environ Radioact 69:225–240

    CAS  Google Scholar 

  • Tirmarche M, Harrison J, Laurier D, Blanchardon E, Paquet F, Marsh J (2012) Risk of lung cancer from radon exposure: contribution of recently published studies of uranium miners. Ann ICRP 41(3–4):368–377

    CAS  Google Scholar 

  • Trevisi R, Risica S, D’Alessandro M, Paradiso D, Nuccetelli C (2012) Natural radioactivity in building materials in the European Union: a database and an estimate of radiological significance. J Environ Radioact 105:11–20

    CAS  Google Scholar 

  • Tufan MÇ, Dişçi T (2013) Natural radioactivity measurements in building materials used in Samsun, Turkey. Radiat Prot Dosim 156(1):87–92

    CAS  Google Scholar 

  • Tuo F, Peng X, Zhou Q, Zhang J (2020) Assessment of natural radioactivity levels and radiological hazards in building materials. Radiat Prot Dosim 188(3):316–321

    CAS  Google Scholar 

  • Turhan Ş, Baykan UN, Şen K (2008) Measurement of the natural radioactivity in building materials used in Ankara and assessment of external doses. J Radiol Prot 28:83–91

    CAS  Google Scholar 

  • Turhan Ş (2009) Radiological impacts of the usability of clay and kaolin as raw material in manufacturing of structural building materials in Turkey. J Radiol Prot 29:75–83

    CAS  Google Scholar 

  • Turhan Ş (2010) Radioactivity levels of limestone and gypsum used as building raw materials in Turkey and estimation of exposure doses. Radiat Prot Dosim 140(4):402–407

    CAS  Google Scholar 

  • Turhan Ş, Arıkan İH, Demirel H, Güngör N (2011) Radiometric analysis of raw materials and end products in the Turkish ceramics industry. Radiat Phys Chem 80(5):620–625

    CAS  Google Scholar 

  • Turhan Ş, Varinlioğlu A (2012) Radioactivity measurement of primordial radionuclides in and dose evaluation from marble and glazed tiles used as covering building materials in Turkey. Radiat Prot Dosim 151(3):546–555

    CAS  Google Scholar 

  • Turhan Ş, Temirci AT, Kurnaz A, Altıkulaç A, Gören E, Karataşlı M, Kırışık R, Hançerlioğulları A (2018) Natural radiation exposure and radon exhalation rate of building materials used in Turkey. Nucl Technol Radiat Prot 33(2):159–266

    CAS  Google Scholar 

  • UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) 2008 (2010) Sources and effects of ionizing radiation. United Nations Scientific Committee on the Effects of Atomic Radiation, United Nations Publication, New York, USA

  • UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) (2000) Sources and effects of ionizingrRadiation. United Nations Publication, New York, USA

  • WHO (World Health Organization) (2009) Handbook on indoor radon: a public health perspective edited by Hajo Zeeb, and Ferid Shannoun. WHO Lirary Cataloguing-in-Publication Data

  • Yapıcı N, Gezer F, Nurlu N, Turha Ş, Ufuktepe Y (2017) Radiological, geochemical, and mineralogical characterization of natural stones used in Turkey. Nucl Technol Radiat Prot 32(3):267–274

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Contributions

M. Karataşlı collected the building samples and prepared the samples for the radioactivity measurements. A. Kurnaz and Ş. Turhan performed the laboratory measurements and analyzed the spectra and done the spectra evaluations and the data analysis including the statistical analysis. Ş. Turhan was a major contributor in writing the manuscript. All authors read and approved the final manuscript.

Corresponding author

Correspondence to Asli Kurnaz.

Ethics declarations

Ethics approval

All analyses were based on previous published studies; thus, no ethical approval consent is required.

Consent to participate

Not applicable.

Consent for publication

All authors have checked the manuscript and have agreed to the publication on ESPR.

Competing interests

The authors declare no competing interests.

Additional information

Responsible Editor: Georg Steinhauser

Publisher’s note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Turhan, ., Kurnaz, A. & Karataşlı, M. Evaluation of natural radioactivity levels and potential radiological hazards of common building materials utilized in Mediterranean region, Turkey. Environ Sci Pollut Res 29, 10575–10584 (2022). https://doi.org/10.1007/s11356-021-16505-7

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11356-021-16505-7

Keywords

Navigation