Abstract
Aerosols from the Fukushima Dai-ichi Nuclear Power Plant accident were collected at the Geological Survey of Japan. The temporal patterns of the 134Cs/137Cs, 136Cs/137Cs, and 132Te/137Cs activity ratios were consistent with expectations based on their half-lives. Those for 131I and 129mTe decreased with some fluctuations. 110mAg/137Cs declined more rapidly than expected and 95Nb/137Cs increased with time. The results suggest that the temporal patterns depended not only on their half-lives but also on many factors such as chemical speciation, the diversity of sources, changes in the temperature and discharge rate from the reactors, and the processes of transport.
Similar content being viewed by others
References
Kanai Y (2012) J Environ Radioact 111:33–37
Kanai Y (2012) Bull Geol Surv Jpn 63:107–118
Doi T, Masumoto K, Toyoda A, Tanaka A, Shibata Y, Hirose K (2013) J Environ Radioact 122:55–62
Amano H, Akiyama M, Chunlei B, Kawamura T, Kishimoto T, Kuroda T, Muroi T, Odaira T, Ohta Y, Takeda K, Watanabe Y, Morimoto T (2012) J Environ Radioact 111:42–52
Haba H, Kanaya J, Mukai H, Kambara T, Kase M (2012) Geochem J 46:271–278
KEK (2011) Radiation monitoring at KEK. http://www.legacy.kek.jp/quake/radmonitor/index-e.html. Accessed 20 Aug 2013
Momoshima N, Sugihara S, Ichikawa R, Yokoyama H (2012) J Environ Radioact 111:28–32
TEPCO (2011) News, Press Release. http://www.tepco.co.jp/en/press/corp-com/release/index-e.html. Accessed 20 Aug 2013
Kanai Y, Saito Y (2011) Bull Geol Surv Jpn 62:357–369
Kanai Y, Doi T, Masumoto K (2013) Bull Geol Surv Jpn 64:139–150
METI (2011) http://www.meti.go.jp/press/2011/06/20110606008/20110606008-2.pdf, http://www.meti.go.jp/press/2011/10/20111020001/20111020001.pdf Accessed 20 Aug 2013
TEPCO (2012) Press Release (May 24, 2012) The estimated amount of radioactive materials released into the air and the ocean caused by Fukushima Daiichi nuclear power station accident due to the Tohoku-Chihou-Taiheiyou-Oki earthquake (as of May 2012) http://www.tepco.co.jp/en/press/corp-com/release/2012/1204659_1870.html, http://www.tepco.co.jp/en/press/corp-com/release/betu12_e/images/120524e0205.pdf, http://www.tepco.co.jp/cc/press/betu12_j/images/120524j0105.pdf. Accessed 20 Aug 2013
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Kanai, Y. Geochemical behavior and activity ratios of Fukushima-derived radionuclides in aerosols at the Geological Survey of Japan, Tsukuba, Japan. J Radioanal Nucl Chem 303, 1405–1408 (2015). https://doi.org/10.1007/s10967-014-3495-1
Received:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s10967-014-3495-1