The determination by an independent method ofP _k electron capture probabilities in¹³³Ba and¹³⁹Ce decays gamma decay of¹³³Ba

Abstract

The electron capture decays of¹³³Ba (10.4 y) and¹³⁹Ce (140 d) were investigated with high resolution Ge(Li) detectors. By x-ray — γ-ray coincidences values of the quantityP _k ω _k ɛ _k for various transitions in the decay of¹³³Ba and¹³⁹Ce are obtained. The factor ω _k ɛ _k was measured independently by means ofK-conversion electron-K x-ray coincidences and was then used to determineP _k , theK-capture probability. The independent measurement of the product ω _k ɛ _k , together with recent accurate values of ω _k , provides a new method for the accurate calibration of semiconductor x-ray detectors. In the decay of¹³⁹Ce, a value ofP _k =0.78±0.03 is found (where the error represents twice the standard deviation) from whichQ _ec =326 ⁺⁷⁰₋₃₀ keV to the¹³⁹La ground-state is found by use of theory. In¹³³Ba decay, values are found ofP _k 1=0.72±0.04 for theEC transition to the 437 keV level in¹³³Cs,P _k 2=0.80±0.07 to the 384 keV level, and from an independent measurement, the ratioP _k 1/P _k 2=0.87±0.07. From these results the ground-state value ofQ _ec =522 ⁺²⁰₋₁₀ keV is derived from theory for¹³³Ba decay. The gamma spectrum of¹³³Ba also was remeasured. From the present gamma intensities and previous conversion electron intensities, new values forK-shell conversion coefficients are obtained. Previously reported γ-rays at 35 and 391 keV are not confirmed.