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Temperature-Stable Dielectric Properties from − 56°C to 248°C in (1 − x)BaTiO3-xBi(Mg0.5Sn0.5)O3 System

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Abstract

(1 − x)BaTiO3-xBi(Mg0.5Sn0.5)O3 [BTBMS, 0.02 ≤ x ≤ 0.12, x represents the amount of Bi(Mg0.5Sn0.5)O3 (mol.%)] ceramics that were prepared by a traditional solid state reaction technique. X-ray diffraction results demonstrated that BTBMS belongs to a homogenous solid solution. The composition with x = 0.1 has the best properties with a stable relative permittivity (εr ~ 2918), the thermal-stability of relative permittivity (Δε/ε25°C ≤ ± 15%) in a large range of temperature from − 56 to 248°C and low dielectric loss (tanδ ≤ 0.025) from − 54 to 125°C. The relaxation in the high temperature region is thermally activated, and the oxygen vacancies may be the ionic charge carriers. Moreover, energy storage efficiency reaches the maximum at x = 0.1.

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Acknowledgments

This study was supported by Natural Science Foundation of China (Nos. 11664008, 11464009 and 61761015), Natural Science Foundation of Guangxi (Nos. 2017GXNSFDA198027 and 2017GXNSFFA 198011) and the Research Start-up Funds Doctor of Guilin University of Technology (No. GUTQD JJ2017133).

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Authors and Affiliations

  1. Collaborative Innovation Center for Exploration of Hidden Nonferrous Metal Deposits and Development of New Materials in Guangxi, Key Laboratory of Nonferrous Materials and New Processing Technology, Ministry of Education, School of Materials Science and Engineering, Guilin University of Technology, Guilin, 541004, China

    Xiaoxia Li, Xiuli Chen, Xiaobin Liu, Xiao Yan, Huanfu Zhou, Gaofeng Liu, Xu Li & Jie Sun

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  1. Xiaoxia Li
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  2. Xiuli Chen
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  3. Xiaobin Liu
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  7. Xu Li
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Correspondence to Xiuli Chen.

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Li, X., Chen, X., Liu, X. et al. Temperature-Stable Dielectric Properties from − 56°C to 248°C in (1 − x)BaTiO3-xBi(Mg0.5Sn0.5)O3 System. J. Electron. Mater. 48, 296–303 (2019). https://doi.org/10.1007/s11664-018-6714-7

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  • DOI: https://doi.org/10.1007/s11664-018-6714-7

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