Abstract
We have achieved first steps toward coherent control of excitonic energy migration in the FMO pigment-protein complex, by combining femtosecond pulse shaping with a feedback loop using an evolutionary algorithm. The experimental conditions achieved, with a rotating sample, a cryostat, and a pulse shaper, are sufficient for closed loop optimizations.
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
References
R. Fenna, B. Matthews, Nature 258, 573, 1975
J. Olson, C. Romano, Biochimica Biophysica Acta 59, 726, 1962
T. Brixner, J. Stenger, H. M. Vaswani, M. Cho, R.E. Blankenship and G. R. Fleming, Nature, 434, 625, 2005
R.S. Judson, H. Rabitz, Phys. Rev. Lett. 68, 1500, 1992
J. L. Herek, W. Wohlleben, R. J. Cogdell, D. Zeidler, M. Motzkus, Nature 417, 533, 2002
B. Brüggemann and V. May, J. Phys. Chem. B 108, 10529, 2004
Author information
Authors and Affiliations
Corresponding author
Editor information
Editors and Affiliations
Rights and permissions
Copyright information
© 2009 Springer-Verlag Berlin Heidelberg
About this paper
Cite this paper
Milder, M.T.W., Brüggemann, B., Miller, M., Herek, J.L. (2009). Coherent Control of the Exciton Dynamics in the FMO Protein. In: Corkum, P., Silvestri, S., Nelson, K., Riedle, E., Schoenlein, R. (eds) Ultrafast Phenomena XVI. Springer Series in Chemical Physics, vol 92. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-95946-5_145
Download citation
DOI: https://doi.org/10.1007/978-3-540-95946-5_145
Published:
Publisher Name: Springer, Berlin, Heidelberg
Print ISBN: 978-3-540-95945-8
Online ISBN: 978-3-540-95946-5
eBook Packages: Physics and AstronomyPhysics and Astronomy (R0)